articleJournal of the American Chemical SocietyApr 10, 2025Closed access

Regulating Enol-to-Keto Tautomerization of Pillararene-Based Conjugated Macrocycle Polymers for H 2 O 2 Photosynthesis

Jilin University · State Key Laboratory of Inorganic Synthesis and Preparative Chemistry · +1 more institution

PubMed
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Abstract

. In-depth investigations reveal that the incorporation of pillararenes enables synergistic catalysis of water oxidation and oxygen reduction reactions and significantly enhances catalyst stability by regulating molecular tautomerization. This work opens new avenues for designing high-performance multifunctional conjugated macrocycle polymers with significant potential for clean energy conversion.

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