Photothermal-Enhanced Anti-SO 2 Performance of a MoWO x /CeO 2 Catalyst in Low-Temperature NH 3 -SCR
University of Science and Technology of China · Chinese Academy of Sciences · +1 more institution
Abstract
Cerium-based catalysts for the selective catalytic reduction of NOx with ammonia (NH3-SCR) face significant challenges in practical applications, particularly their poor low-temperature activity and susceptibility to SO2 poisoning. In this study, photothermal catalysis was innovatively applied to the NH3-SCR reaction over MoWOx/CeO2 catalysts, achieving remarkable improvements in the low-temperature performance and SO2 resistance. Under photothermal conditions, the catalyst maintained NOx conversion above 90% at 200 °C, even in the presence of 250 ppm of SO2. Comprehensive characterization revealed that light irradiation significantly enhanced the formation of oxygen vacancies on the catalyst surface and…
Citation impact
- FWCI
- 24.38
- Percentile
- 100%
- References
- 43
Authors
10- XHXinyu Han
University of Science and Technology of China, Chinese Academy of Sciences
- LJLiangliang Jiang
University of Calgary
- ZZZeshu Zhang
University of Science and Technology of China, Chinese Academy of Sciences
- KLKaijie LiuCorresponding
University of Science and Technology of China, Chinese Academy of Sciences
- MBMengyao Bian
University of Science and Technology of China, Chinese Academy of Sciences
Topics & keywords
- Catalysis
- NOx
- Selective catalytic reduction
- Adsorption
- Photothermal therapy
- Chemistry
- Ammonia
- Cerium oxide
Funding
- DTDouble Thousand Plan of Jiangxi ProvinceAward: jxsq2020101047
- NNNational Natural Science Foundation of ChinaAwards: 22176185, 22472178, 22302206, 22072141, 52304429, 22208270
- YIYouth Innovation Promotion Association of the Chinese Academy of SciencesAward: 2018263
- KRKey Research and Development Program of Jiangxi ProvinceAward: 20232BBG70012
- SFScience Fund for Distinguished Young Scholars of Jiangxi ProvinceAward: 20232ACB213004
- NKNational Key Research and Development Program of ChinaAward: 2022YFB3504200
- GIGanjiang Innovation Academy, Chinese Academy of SciencesAwards: E355C001, E32PF00121