Determination of Mn Valence States in Nanocatalysts During Sustainable Syngas Conversion
Frontier Science Foundation · Carbon180 · +5 more institutions
Abstract
Constructing structure–activity relationships (SAR) between nanocatalysts under reactive atmospheres makes them indispensable for chemical synthesis, energy transformation, and environmental remediation. However, this structure sensitivity remains ambiguous for metals/metal oxides due to dynamic changes in metal valences under a reductive atmosphere. Herein, this study delves into the complexities of Mn-based nanocatalysts, focusing on the impact of the Mn valence state in a test reaction converting sustainable syngas to aromatics-a process highly sensitive to the catalyst’s redox environment and active site characteristics. We conducted a thorough SAR analysis and discovered a direct correlation between the…
Citation impact
- FWCI
- 37.17
- Percentile
- 100%
- References
- 74
Authors
11Topics & keywords
- Chemistry
- Nanomaterial-based catalyst
- Syngas
- Valence (chemistry)
- Catalysis
- Organic chemistry
- Responsible consumption and production