articleChemistry of MaterialsJan 7, 2026HYBRID OA

Operando Synchrotron-Based Fourier Transform Infrared Microspectroscopy of Metal-Ion Organic Battery Materials

Institut de Ciència de Materials de Barcelona · Madrid Institute for Advanced Studies · +7 more institutions

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Abstract

SR-μFTIR microspectroscopy can be applied to the study of electrode materials, electrolytes, and electrode-electrolyte interfaces. It is especially valuable for the elucidation of reaction mechanisms taking place in noncrystalline and/or lightweight element-based electrodes, such as organic electrode materials. Herein, we show how a simple modification of the commercially available ECC-Opto-Std (ELCELL) cell allows unraveling the potential of operando SR-μFTIR microspectroscopy for investigating organic electrodes. This setup is applied to study the reaction mechanism of polyimide derived from 1,4,5,8-naphthalenetetracarboxylic dianhydride (NTCDA) in lithium, sodium, and calcium cells. During the…

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